Trends and perspectives in per-and polyfluorinated alkyl substances (PFASs) determination: Faster and broader

Ke Gao; Yu Chen; Qiao Xue; Jie Fu; Kehan Fu; Jianjie Fu; Aiqian Zhang; Zongwei CAI; Guibin Jiang

doi:10.1016/j.trac.2020.116114

Trends and perspectives in per-and polyfluorinated alkyl substances (PFASs) determination: Faster and broader

Ke Gao
, Yu Chen
, Qiao Xue
, Jie Fu
, Kehan Fu
, Jianjie Fu^*
, Aiqian Zhang
, Zongwei CAI
, Guibin Jiang

^*Corresponding author for this work

Department of Chemistry

Research output: Contribution to journal › Review article › peer-review

61 Citations (Scopus)

Abstract

Per-and polyfluorinated alkyl substances (PFASs) have been in the spotlight due to their pervasiveness, environmental persistence, bioaccumulation/magnification potential, and possible ecological and health risks. However, the detection of PFASs in the environment represents a longstanding technical challenge. Research on the environmental behavior and risk assessment of PFASs has greatly increased due to advancements in modern analytical methods. Numerous PFASs with varied applications and physicochemical properties are in use, which makes the integrated PFAS analysis challenging. Great advancements in sample pretreatment and instrumental analysis for PFASs have been made since the 2000s, allowing faster and broader PFAS determination. The concern over PFASs in the environment has gradually extended from legacy perfluoroalkyl acids (PFAAs) to novel PFASs. This review outlines the trends and challenges in PFAS determination and proposes perspectives for future PFAS analysis.

Original language	English
Article number	116114
Journal	TrAC - Trends in Analytical Chemistry
Volume	133
DOIs	https://doi.org/10.1016/j.trac.2020.116114
Publication status	Published - Dec 2020

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This output contributes to the following UN Sustainable Development Goals (SDGs)

SDG 3 Good Health and Well-being

User-Defined Keywords

High resolution mass spectrometry
Instrumental analysis technique
Non-targeted analysis
Per-and polyfluorinated alkyl substances (PFASs)
Sample preparation

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10.1016/j.trac.2020.116114

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@article{512bc54bd7ed4c2798326e888984f22e,

title = "Trends and perspectives in per-and polyfluorinated alkyl substances (PFASs) determination: Faster and broader",

abstract = "Per-and polyfluorinated alkyl substances (PFASs) have been in the spotlight due to their pervasiveness, environmental persistence, bioaccumulation/magnification potential, and possible ecological and health risks. However, the detection of PFASs in the environment represents a longstanding technical challenge. Research on the environmental behavior and risk assessment of PFASs has greatly increased due to advancements in modern analytical methods. Numerous PFASs with varied applications and physicochemical properties are in use, which makes the integrated PFAS analysis challenging. Great advancements in sample pretreatment and instrumental analysis for PFASs have been made since the 2000s, allowing faster and broader PFAS determination. The concern over PFASs in the environment has gradually extended from legacy perfluoroalkyl acids (PFAAs) to novel PFASs. This review outlines the trends and challenges in PFAS determination and proposes perspectives for future PFAS analysis.",

keywords = "High resolution mass spectrometry, Instrumental analysis technique, Non-targeted analysis, Per-and polyfluorinated alkyl substances (PFASs), Sample preparation",

author = "Ke Gao and Yu Chen and Qiao Xue and Jie Fu and Kehan Fu and Jianjie Fu and Aiqian Zhang and Zongwei CAI and Guibin Jiang",

note = "Funding Information: This study was jointly supported by the National Key Research and Development Program of China ( 2018YFF0214801-02 ), National Natural Science Foundation of China ( 21976188 , 22022611 , 91743204 , 21677168 ) and the Youth Innovation Promotion Association of CAS ( 2018052 ). Funding Information: This study was jointly supported by the National Key Research and Development Program of China (2018YFF0214801-02), National Natural Science Foundation of China (21976188, 22022611,91743204, 21677168) and the Youth Innovation Promotion Association of CAS (2018052).",

year = "2020",

month = dec,

doi = "10.1016/j.trac.2020.116114",

language = "English",

volume = "133",

journal = "TrAC - Trends in Analytical Chemistry",

issn = "0165-9936",

publisher = "Elsevier B.V.",

}

TY - JOUR

T1 - Trends and perspectives in per-and polyfluorinated alkyl substances (PFASs) determination

T2 - Faster and broader

AU - Gao, Ke

AU - Chen, Yu

AU - Xue, Qiao

AU - Fu, Jie

AU - Fu, Kehan

AU - Fu, Jianjie

AU - Zhang, Aiqian

AU - CAI, Zongwei

AU - Jiang, Guibin

N1 - Funding Information: This study was jointly supported by the National Key Research and Development Program of China ( 2018YFF0214801-02 ), National Natural Science Foundation of China ( 21976188 , 22022611 , 91743204 , 21677168 ) and the Youth Innovation Promotion Association of CAS ( 2018052 ). Funding Information: This study was jointly supported by the National Key Research and Development Program of China (2018YFF0214801-02), National Natural Science Foundation of China (21976188, 22022611,91743204, 21677168) and the Youth Innovation Promotion Association of CAS (2018052).

PY - 2020/12

Y1 - 2020/12

N2 - Per-and polyfluorinated alkyl substances (PFASs) have been in the spotlight due to their pervasiveness, environmental persistence, bioaccumulation/magnification potential, and possible ecological and health risks. However, the detection of PFASs in the environment represents a longstanding technical challenge. Research on the environmental behavior and risk assessment of PFASs has greatly increased due to advancements in modern analytical methods. Numerous PFASs with varied applications and physicochemical properties are in use, which makes the integrated PFAS analysis challenging. Great advancements in sample pretreatment and instrumental analysis for PFASs have been made since the 2000s, allowing faster and broader PFAS determination. The concern over PFASs in the environment has gradually extended from legacy perfluoroalkyl acids (PFAAs) to novel PFASs. This review outlines the trends and challenges in PFAS determination and proposes perspectives for future PFAS analysis.

AB - Per-and polyfluorinated alkyl substances (PFASs) have been in the spotlight due to their pervasiveness, environmental persistence, bioaccumulation/magnification potential, and possible ecological and health risks. However, the detection of PFASs in the environment represents a longstanding technical challenge. Research on the environmental behavior and risk assessment of PFASs has greatly increased due to advancements in modern analytical methods. Numerous PFASs with varied applications and physicochemical properties are in use, which makes the integrated PFAS analysis challenging. Great advancements in sample pretreatment and instrumental analysis for PFASs have been made since the 2000s, allowing faster and broader PFAS determination. The concern over PFASs in the environment has gradually extended from legacy perfluoroalkyl acids (PFAAs) to novel PFASs. This review outlines the trends and challenges in PFAS determination and proposes perspectives for future PFAS analysis.

KW - High resolution mass spectrometry

KW - Instrumental analysis technique

KW - Non-targeted analysis

KW - Per-and polyfluorinated alkyl substances (PFASs)

KW - Sample preparation

UR - https://www.scopus.com/pages/publications/85096352913

U2 - 10.1016/j.trac.2020.116114

DO - 10.1016/j.trac.2020.116114

M3 - Review article

AN - SCOPUS:85096352913

SN - 0165-9936

VL - 133

JO - TrAC - Trends in Analytical Chemistry

JF - TrAC - Trends in Analytical Chemistry

M1 - 116114

ER -

Trends and perspectives in per-and polyfluorinated alkyl substances (PFASs) determination: Faster and broader

Abstract

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