Intensity dependence of intramolecular interference from a full quantum analysis of high-order harmonic generation

Y. J. Chen; J. Liu; Bambi Hu

doi:10.1103/PhysRevA.79.033405

Intensity dependence of intramolecular interference from a full quantum analysis of high-order harmonic generation

Y. J. Chen, J. Liu, Bambi Hu

Research output: Contribution to journal › Journal article › peer-review

29 Citations (Scopus)

Abstract

We develop a numerical scheme to investigate the high-order harmonic generation (HHG) in intense laser-matter interactions. We represent the time-dependent wave function in the basis of the eigenstates of the field-free Hamiltonian and trace its temporal evolution. Our full quantum simulations reveal that continuum electrons with a broad energy distribution contribute equally to one harmonic and the excited state also plays an important role in the molecular HHG. These results imply a laser-intensity-dependent picture of intramolecular interference in the HHG.

Original language	English
Article number	033405
Journal	Physical Review A
Volume	79
Issue number	3
DOIs	https://doi.org/10.1103/PhysRevA.79.033405
Publication status	Published - 13 Mar 2009

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

Access to Document

10.1103/PhysRevA.79.033405

Cite this

@article{72f0cb21476f4e9e8a6de41dacc4439b,

title = "Intensity dependence of intramolecular interference from a full quantum analysis of high-order harmonic generation",

abstract = "We develop a numerical scheme to investigate the high-order harmonic generation (HHG) in intense laser-matter interactions. We represent the time-dependent wave function in the basis of the eigenstates of the field-free Hamiltonian and trace its temporal evolution. Our full quantum simulations reveal that continuum electrons with a broad energy distribution contribute equally to one harmonic and the excited state also plays an important role in the molecular HHG. These results imply a laser-intensity-dependent picture of intramolecular interference in the HHG.",

author = "Chen, {Y. J.} and J. Liu and Bambi Hu",

note = "Publisher copyright: {\textcopyright} 2009 American Physical Society",

year = "2009",

month = mar,

day = "13",

doi = "10.1103/PhysRevA.79.033405",

language = "English",

volume = "79",

journal = "Physical Review A",

issn = "2469-9926",

publisher = "American Physical Society",

number = "3",

}

TY - JOUR

T1 - Intensity dependence of intramolecular interference from a full quantum analysis of high-order harmonic generation

AU - Chen, Y. J.

AU - Liu, J.

AU - Hu, Bambi

PY - 2009/3/13

Y1 - 2009/3/13

N2 - We develop a numerical scheme to investigate the high-order harmonic generation (HHG) in intense laser-matter interactions. We represent the time-dependent wave function in the basis of the eigenstates of the field-free Hamiltonian and trace its temporal evolution. Our full quantum simulations reveal that continuum electrons with a broad energy distribution contribute equally to one harmonic and the excited state also plays an important role in the molecular HHG. These results imply a laser-intensity-dependent picture of intramolecular interference in the HHG.

AB - We develop a numerical scheme to investigate the high-order harmonic generation (HHG) in intense laser-matter interactions. We represent the time-dependent wave function in the basis of the eigenstates of the field-free Hamiltonian and trace its temporal evolution. Our full quantum simulations reveal that continuum electrons with a broad energy distribution contribute equally to one harmonic and the excited state also plays an important role in the molecular HHG. These results imply a laser-intensity-dependent picture of intramolecular interference in the HHG.

UR - http://www.scopus.com/inward/record.url?scp=63149144496&partnerID=8YFLogxK

U2 - 10.1103/PhysRevA.79.033405

DO - 10.1103/PhysRevA.79.033405

M3 - Journal article

AN - SCOPUS:63149144496

SN - 2469-9926

VL - 79

JO - Physical Review A

JF - Physical Review A

IS - 3

M1 - 033405

ER -

Intensity dependence of intramolecular interference from a full quantum analysis of high-order harmonic generation

Abstract

UN SDGs

Access to Document

Other files and links

Fingerprint

Cite this